Keywords

molten salt, rotating eletrodes, electrochemistry

Abstract

In this paper, we describe and validate a custom apparatus for performing high-speed (250-3,500 rpm) rotating electrode and dilatometer density experiments in molten salts. The reported details can aid in decreasing the difficulty and increasing the quality of such experiments. We discuss the design challenges and the solutions identified. We investigate methods for accurately measuring the solution resistance using electrochemical impedance spectroscopy (EIS), calculating the working electrode area using cyclic voltammetry (CV), and measuring the mass transfer-limited current of rotating electrodes using a series of chronoamperometry (CA) pulses. We further demonstrate the efficacy of our methods in producing accurate results.

Original Publication Citation

Fuller, R., Cluff, E., Mercado, E., Mejia, C., & Rappleye, D. (2025). Methods for Rotating Electrodes in High-Temperature Molten Salts. Journal of The Electrochemical Society, 172(4), 043510. https://doi.org/10.1149/1945-7111/adcaef

Document Type

Peer-Reviewed Article

Publication Date

2025-04-23

Publisher

Journal of The Electrochemical Society

Language

English

College

Ira A. Fulton College of Engineering

Department

Chemical Engineering

University Standing at Time of Publication

Assistant Professor

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